Coulomb-correlated electron number states in a transmission electron microscope beam

نویسندگان

چکیده

We demonstrate the generation of Coulomb-correlated pair, triple and quadruple states free electrons by femtosecond photoemission from a nanoscale field emitter inside transmission electron microscope. Event-based spectroscopy allows spatial spectral characterization ensemble emitted each laser pulse. identify distinctive energy momentum correlations arising acceleration-enhanced interparticle exchange, revealing strong few-body Coulomb interactions at an scale about two electronvolts. State-sorted beam caustics show discrete increase in virtual source size longitudinal shift for few-electron states, associated with transverse correlations. observe field-controllable antibunching, attributed primarily to deflection. The pronounced characteristics these number allow filtering schemes that control statistical distribution pulse charge. In this way, fraction specific can be actively suppressed or enhanced, facilitating preparation highly non-Poissonian beams microscopy lithography, including future heralding correlated multi-electron probing.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Beam-induced motion of adatoms in the transmission electron microscope.

Equations governing the elastic scattering of electrons are applied to the knock-on displacement of atoms along a substrate, yielding analytical expressions for the surface-translation energy, threshold incident energy, and displacement rate. For a surface perpendicular to the incident beam, scattering angles around 90° contribute most to the kinetic energy of surface atoms. Tilting the specime...

متن کامل

Isotope analysis in the transmission electron microscope

The Ångström-sized probe of the scanning transmission electron microscope can visualize and collect spectra from single atoms. This can unambiguously resolve the chemical structure of materials, but not their isotopic composition. Here we differentiate between two isotopes of the same element by quantifying how likely the energetic imaging electrons are to eject atoms. First, we measure the dis...

متن کامل

Electron microscopy’s multi-tool: the Scanning Transmission Electron Microscope

A dedicated Scanning Transmission Electron Microscope is ideally coupled with the energy dispersive x-ray and electron energy loss spectroscopies to obtain information about the chemical composition, morphology and electronic structure on the nanoscale. With several signals being available simultaneously with the pass of a subnanometre-sized beam, this instrument can answer questions from a bro...

متن کامل

Parallel electron-beam-induced deposition using a multi-beam scanning electron microscope

Lithography techniques based on electron-beam-induced processes are inherently slow compared to light lithography techniques. The authors demonstrate here that the throughput can be enhanced by a factor of 196 by using a scanning electron microscope equipped with a multibeam electron source. Using electron-beam induced deposition with MeCpPtMe3 as a precursor gas, 14 14 arrays of Pt-containing ...

متن کامل

Precession Electron Diffraction in the Transmission Electron Microscope: electron crystallography and orientational mapping

Precession electron diffraction (PED) is a hollow cone non-stationary illumination technique for electron diffraction pattern collection under quasikinematical conditions (as in X-ray Diffraction), which enables “ab-initio” solving of crystalline structures of nanocrystals. The PED technique is recently used in TEM instruments of voltages 100 to 300 kV to turn them into true electron diffractom...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: Nature Physics

سال: 2023

ISSN: ['1745-2473', '1745-2481']

DOI: https://doi.org/10.1038/s41567-023-02067-7